No, there's no way to easily do that, but I have a work-around for you.
Say for example, in your design (most likely album.php) you want the main picture in the middle of the page, then a thumbnail of the previous image to the left of the main picture and a preview of the next image to the right of the main picutre.
What you can do is have people set
`$conf['images_per_page']`
to three (the preview on the left, the middle picture, and the preview on the right).
Then inside your image [b]while loop[/b] you can just have a conditional statement that says that if it's the middle image, use a getCustomImageURL() with a larger size.